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j.nimb.2015.09.018.pdf | 331.35 kB | Adobe PDF | 見る/開く |
タイトル: | Effects of radical scavengers on aqueous solutions exposed to heavy-ion irradiation using the liquid microjet technique |
著者: | Nomura, Shinji Tsuchida, Hidetsugu https://orcid.org/0000-0001-9989-1074 (unconfirmed) Furuya, Ryousuke Miyahara, Kento Majima, Takuya https://orcid.org/0000-0003-2804-1915 (unconfirmed) Itoh, Akio |
著者名の別形: | 土田, 秀次 |
キーワード: | Radical scavenger effects Liquid materials Fast heavy-ion irradiation |
発行日: | 15-Dec-2015 |
出版者: | Elsevier B.V. |
誌名: | Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms |
巻: | 365 |
開始ページ: | 611 |
終了ページ: | 615 |
抄録: | The effects of the radical scavenger ascorbic acid on water radiolysis are studied by fast heavy-ion irradiation of aqueous solutions of ascorbic acid, using the liquid microjet technique under vacuum. To understand the reaction mechanisms of hydroxyl radicals in aqueous solutions, we directly measure secondary ions emitted from solutions with different ascorbic acid concentrations. The yield of hydronium secondary ions is strongly influenced by the reaction between ascorbic acid and hydroxyl radicals. From analysis using a simple model considering chemical equilibria, we determine that the upper concentration limit of ascorbic acid with a radical scavenger effect is approximately 70 μM. |
著作権等: | © 2015. This manuscript version is made available under the CC-BY-NC-ND 4.0 license http://creativecommons.org/licenses/by-nc-nd/4.0/ The full-text file will be made open to the public on 15 December 2017 in accordance with publisher's 'Terms and Conditions for Self-Archiving'. This is not the published version. Please cite only the published version. この論文は出版社版でありません。引用の際には出版社版をご確認ご利用ください。 |
URI: | http://hdl.handle.net/2433/203604 |
DOI(出版社版): | 10.1016/j.nimb.2015.09.018 |
出現コレクション: | 学術雑誌掲載論文等 |
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