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Title: High-order harmonic generation from hybrid organic-inorganic perovskite thin films
Authors: Hirori, Hideki  kyouindb  KAKEN_id  orcid (unconfirmed)
Xia, Peiyu
Shinohara, Yasushi
Otobe, Tomohito
Sanari, Yasuyuki
Tahara, Hirokazu  kyouindb  KAKEN_id  orcid (unconfirmed)
Ishii, Nobuhisa
Itatani, Jiro
Ishikawa, L., Kenichi
Aharen, Tomoko
Ozaki, Masashi
Wakamiya, Atsushi  kyouindb  KAKEN_id  orcid (unconfirmed)
Kanemitsu, Yoshihiko  kyouindb  KAKEN_id  orcid (unconfirmed)
Author's alias: 廣理, 英基
佐成, 晏之
田原, 弘量
若宮, 淳志
金光, 義彦
Issue Date: Apr-2019
Publisher: AIP Publishing
Journal title: APL Materials
Volume: 7
Issue: 4
Thesis number: 041107
Abstract: The generation of high-order harmonics from hybrid organic–inorganic perovskites (HOIPs) is demonstrated by the excitation with a strong mid-infrared laser pulse. We prepare three types of HOIP polycrystalline thin film samples by solution processes (MAPbX₃; MA = CH₃NH₃⁺; X = I, Br, Cl). The high-order harmonics from the sample (MAPbBr₃) are more than tenfold stronger than those from the well-studied GaSe crystal despite their comparable bandgap energies, implying that the stronger band-to-band transition of the HOIPs causes the higher yields.
Rights: © 2019 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution (CC BY) license (
DOI(Published Version): 10.1063/1.5090935
Appears in Collections:Journal Articles

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