Ionization and acceleration of multiply charged gold ions in solid film irradiated by high intensity laser

Abstract

In this paper, we present the mechanisms of ionization of a thin gold film irradiated by a high-intensity, short-pulse laser in the range of I=10²⁰⁻²² W/cm² and the associated acceleration of multiply charged gold ions. A numerical one-dimensional simulation using an extended particle-in-cell code, which includes atomic and collisional relaxation processes, indicates that two types of acceleration, hole-boring radiation pressure acceleration (RPA) and target normal sheath acceleration (TNSA), contribute to the generation of highly charged ions with kinetic energies on the order of 10 MeV/u. In each acceleration, a longitudinal electrostatic field excited by different mechanisms dominantly ionizes atoms to higher charge states and accelerates them to the vacuum region from the rear surface, which is opposite the front surface irradiated by the laser field. The field ionization process dominantly ionizes high energy ions to the high charge state, while a large number of ions with energy <1 MeV/u are ionized by an electron impact ionization process. In TNSA, a multiply charged ion generated at the rear surface is accelerated to the maximum energy although the ion with the highest charge state is generated at the front surface in RPA. However, the existence of contamination, such as water vapor, suppresses the ion energy of TNSA to less than that of RPA since the sheath field readily accelerates the protons and oxygen prior to the acceleration of the gold ions. Our derived theoretical scaling describes the maximum ion energy for each charge state in the cases with and without contamination using the relationship between the longitudinal electrostatic field profile near the rear surface and the classical tunnel field ionization model.